Phew! I've added the women! I know it was a long time in coming, and this is nowhere near a comprehensive site (check the links for more resources) but I hope it's a useful one. Right now it's only about half way updated, so please don't panic if nothing works or you can't find someone...
To check seiyuu by specific series (those in our harem, organized pretty much in alphabetical order) go to the Seiyuu by Series page.
Akaida Yoshihiko
Nishikada Soujiro - Hana Yori Dango
Amano Yuri
Peau d'Roquefort - Hyper Police
Teela - Megami Kouhousei
Yukimura Keiko - Yuu Yuu Hakusho
Ifurita - El Hazard
Kamishiru Miiru - Fushigi Yuugi (OVA)
Ohri - Gestalt
Shouta - Ayashi no Ceres
Aogiri Suzumi - Ayashi no Ceres
Blue - Wolf's Rain
Kurosaki Hisoka - Yami no Matsuei
Canna Nobutoshi Tasuki - Fushigi Yuugi
Gabriel - Tenshi ni Narumon
Mido Ban - GetBackers
Naria, Eries-Hime - Tenkuu no Escaflowne
Araki Kae
Yuuki Miaka - Fushigi Yuugi
Asano Mayumi
Arachne - Angel Sanctuary
Parn - Record of Lodoss (TV)
Kuwabara Kazuma - Yuu Yuu HakushoDi Amon-Hakushaku - Bastard!!
Chiba Susumu
Rosiel - Angel Sanctuary
Hiead Gner - Megami Kouhousei
Noroi - Recca no Honoo
Nakago - Fushigi Yuugi
Sakurazuku Seishirou - X
Mikage Aki - Ayashi no Ceres
Million Knives - Trigun
Genda Tessho
Balgus - Tenkuu no EscaflowneNinja Master Gara - Bastard!!
Dan Dastun - Big O
Toguro otooto - Yuu Yuu Hakusho
General Adon - Berserk
Jebra-taicho - Record of Lodoss (OVA)
Orson - Record of Lodoss (OAV)Hayashibara MegumiAshram - Record of Lodoss (TV)
G - Gestalt
Shion - Please Save My Earth
Nicholas D. Wolfwood - Trigun
Muraki Kazutaka - Yami no Matsuei
Faye Valentine - Cowboy BebopKiritake Yuka (Aquila) - Jikuu Tensho Nazca
Tira Misu - Bakuretsu Hunter
Saotome Ranma (female) - Ranma 1/2
Canal Volfeed - Lost Universe
Seta Soujiro - Rurouni KenshinHiramatsu AkikoMama - Tenshi ni Narumon
Tendo Akane - Ranma 1/2
Kikyo - Inu-Yasha
Kirisawa Fuuko - Recca no HonooHisakawa AyaHelena - Hellsing
Tsubaki - Rurouni Kenshin
Kagurazake Miyabe - Ai Yori Aoshi
Hinoto - X TVSohma Yuki - Fruits Basket
Skuld - Aa! Megami-sama!
Nakajima Yoko - Juuni Kokki
Rem Saverem - Trigun
Taata - Magic Knight Rayearth
Orson - Record of Lodoss (TV)Horie YuiGowa Yushiro - Gasaraki
Ohkuma Daigoru - Rurouni Kenshin
Hikitsu - Fushigi Yuugi
Hiei - Yuu Yuu Hakusho
Link - Legend of Zelda (N64)
Honda Tohru - Fruits BasketFujimiya Aya-chan - Weiß Kreuz
Lei Lin - Samurai: Hunt for the Sword
Hanabishi Kaoru - Ai Yori AoshiFutoin Katsuki - GetBackers
Kusanagi Kei - Onegai Sensei
Kazuma - Scryed
Son Goku - Gensomaden Saiyuki
Kane Blueriver - Lost Universe
Ietomi Yoji
Aoike Kazuya - Hana Yori DangoIizuka Mayumi
Nakatomi Nanaka - Mahou Tsukai Tai!Miruru - Tenshi ni Narumon
Kaori - Weiß Kreuz (OVA)
Cleo Everlasting - Majutsushi Orphen
Millerna-hime - Tenkuu no Escaflowne
Uchida Yukari - Tenkuu no Escaflowne
Sora - Tenkuu no Escaflowne (movie)
Hiko Seijuro - Rurouni KenshinKing Kashue - Record of Lodoss (OAV)
Hermes - Heroic Legend of Arslan
Daryun - Heroic Legend of ArslanInoue KikukoYuki Eiri - Gravitation
Hatori - Fruits Basket
Belldandy - Aa! Megami-sama!Birman - Wei Kreuz
Rune Venus - El Hazard
Kazami Mizuho - Onegai Sensei
Kazuma - Fruits BasketIkura KazueYamanami Keisuke - Peace Maker Kurogane
Ashura - RG VedaImai YukaCarmine - Gestalt
Volcan - Majutsushi Orphen
Uotani Arisa - Fruits BasketInaho Hitomebore - Master of Mosquiton
Kitamura Suzu - Peace Maker Kurogane
Hanafusa Miren - Samurai: Hunt for the Sword
Michael - Tenshi ni NarumonCho Hakkai - Gensomaden Saiyuki
Judeau - Berserk
Ren Shigyou - Fushigi Yuugi OVA
Mitsukake - Fushigi YuugiIshino RyuuzouFujisawa-sensei - El Hazard
Tommy-kun - Hyper PoliceIshizuka UnshoChang Wufei - Gundam Wing
Jet Black - Cowboy BebopB.D. (Brilliant Dynamites) Neon - Trigun
Quent Yaiden - Wolf's Rain
Kuukai - Recca no Honoo
Peter Ferguson - Hellsing
Itou Kentaru
Aoi Jun - Martian Successor Nadesico
Geisel - Weiß Kreuz: Glühen
Minamio - Recca no Honoo
Aogiri Yuuhi - Ayashi no Ceres Itou Miki
Shoen - Weiß KreuzMagami A-ko - Project A-ko
Nova - Magic Knights Rayearth
Sumeragi Hokuto - Tokyo Babylon
Tomite - Fushigi YuugiIwao JunkoAida Kensuke - Neon Genesis Evangelion
Taki Ryuichi - Nightwalker
Mizuhara Makoto - El Hazard
Julius - Trigun
Ceres - Ayashi no CeresAikawa Akane - Mahou Tsukai Tai!
Yukishiro Tomoe - Rurouni Kenshin
Monou Kotori - X the Movie
Tanaka-sensei - Kodomo no OmochaKakazu YumiKaneda - Akira
Dispell-sama - Tenshi ni Narumon
Mikage Aya - Ayashi no CeresDita Liebely - Vandread
Fujimura Leena - Megami Kouhousei
Ashram - Record of Lodoss (OAV)Kasahara Hiroko
Hououji Fuu - Magic Knight RayearthKatsuki MasakoMagdalia Sayo - Rurouni Kenshin
Zakuro - Juubei NinpuchoKawakami TomokoPharangese - Arslan Senki
Hell - Weiß Kreuz
Noelle - Tenshi ni NarumonKawamura MariaUtena - Revolutionary Girl Utena
Kazusa - Yami no Matsuei
Asuka's mother - Neon Genesis EvangelionKawasumi AyakoChida Mamiya - Shoujo Kakumei Utena
Naga - Slayers
Mudo Sara - Angel SanctuaryKikuchi MasamiSakuraba Aoi - Ai Yori Aoshi
Herikawa Koishi - Onegai Sensei
Mayura - Samurai: Hunt for the sword
Melfina - Outlaw Star
Sara - Tenshi ni Narumon
Masaki Tenchi - Tenchi MuyoKingetsu MamiMorisato Keiichi - Aa! Megami-sama!
Higashiyama Ryuzaburou - Rurouni Kenshin
Lars - Bastard!!
Sensei - Tenshi ni NarumonKonishi HirokoDjinn (female) - Gokudo-kun Manyuuki
Miharu - Gasaraki
Sawanoguchi Sae - Mahou Tsukai Tai!Silky - Tenshi ni Narumon
Mirei - Tenchi Muyo
Konishi Katsuyuki
Tooya - Ayashi no CeresOnime no Kyo - Samurai Deeper Kyo
Mibu Kyoshiro - Samurai Deeper Kyo
Riui - Mahou Senshi Riui
Togepei - PokemonMenchi - Excel Saga
Aizenmyoh - RG Veda
Dryden Fassa - Tenkuu no EscaflowneKoyama MamiLantis - Magic Knight Rayearth
Papa - Tenshi ni Narumon
Persia - Weiß Kreuz
Sol Zagato - Magic Knight Rayearth
Tamura - Please Save My Earth
Karen Kasumi - X the MovieKei - Akira
Aoba Shigeru - Neon Genesis EvangelionFujimiya Aya - Weiß Kreuz
Hotohori - Fushigi Yuugi
Pulse - Twin Signal
Daisuke - Ranma 1/2
Ilpalazzo-sama - Excel Saga
Kira Sakuya - Angel Sanctuary
Aburatsubo Ayanojo - Mahou Tsukai Tai!
Melrain - Heroic Legend of Arslan
Tate Masanari - Jikuu Tenshou Nazca
Olivier - Gestalt
Sakurazuka Seishirou - Tokyo Babylon
Zechs Merquise/Millard peacecraft - Gundam Wing
Koganei Kaoru - Recca no Honou
Parn - Record of Lodoss (OAV)Kuwashima HoukoKougaiji - Gensomaden Saiyuki
Sango - Inu-YashaMadono MitsuakiMisumaru Yurika - Nadesico
Philia - Slayers Try
Yatouji Satsuki - X
Marron Glace - Bakuretsu HunterMatsumoto RicaJoker - Recca no Honoo
Gatty (Ryuugekitai) - Tenkuu no Escaflowne
Sorata - X TV
Emishi Haruki - GetBackers
Kite - TrigunSatoshi (Ash) - Pokemon
Fanieta - Vandread
Nataku - X the Movie
Matsumoto Yasunori
Gourry Gabriev - SlayersYami o Makumono (he who strews darkness) - Lost Universe
Paul Wan - GetBackers
Nakano Hiroshi - Gravitation
Matsuno Taiki
Beshimi - Rurouni KenshinMiguel Lavariel - Tenkuu no Escaflowne
Kouga - Inu-Yasha
Mikagami Tokiya - Recca no HonouHeero Yuy - Gundam Wing
Shazan - Gestalt
Schuldig - Weiß Kreuz
Zelgadis - Slayers
Ryohou - Scryed
Rail Claymore - Lost Universe
Tamahome - Fushigi Yuugi
Allen Schezar- Tenkuu no EscaflowneMinaguchi YukoSusumu Amano - Tenkuu no Escaflowne
Kodou Youji - Weiß Kreuz
Katan - Angel Sanctuary
Tsuzuki Asato - Yami no Matsuei
Yuuki Keisuke - Fushigi Yuugi
Yaone - Gensomaden SaiyukiMinami OmiHinoto - X the Movie
Eros - Tenshi ni NarumonMitsuishi KotonoHyatt - Excel Saga
Hoshino Ruri - Nadesico
Majik - Majutsushi Orphen
Kage Houshi - Recca no HonooMiyamura YukoExcel - Excel Saga
Fonne Valkyrie - Hyper Police
Sohma Kagura - Fruits Basket
Shunfaa - Gensomaden Saiyuki
Murase Asuka/Neu - Weiß Kreuz
Yatouji Satsuki - X the Movie
Sasahara Natsuki - Hyper PoliceMizutani YoukoCaska - Berserk
Kurai - Angel Sanctuary
Sohryuu Asuka Langley - Neon Genesis Evangelion
Takatsuki Toki - Rurouni Kenshin
Chocolate Misu - Bakuretsu HunterGreat Will of the Universe - Excel Saga
Mizutani Mihoshi - Tenchi Muyo
Tsume - Wolf's Rain
Miyamoto Mitsuru
Hubb Lebowski - Wolf's RainSohma Ayame - Fruits Basket
Roger Smith, the Negotiator - Big O
Slayn - Record of Lodoss War TV
Kiba - Wolf's Rain
Doumyoji Tsukasa - Hana Yori Dango
Sumeragi Subaru - XKamoshita Yuusuke - Tenshi ni Narumon
Mimisaka Akira - Hana Yori Dango
Ogura Jinpachi - Please Save My EarthHuascar - Jikuu Tenshou Nazca
Griffith - Berserk
Tatsumi Seiichirou - Yami no Matsuei
Iwata - Excel SagaCecil - Record of Lodoss TV
Ginji - GetBackers
Orphen - Majutsushi Orphen
Luck Breed (Tears of an Angel-Ep.10) - Nightwalker
Takeoka Shinjuro - Samurai: Hunt for the Sword
Raphael - Tenshi ni Narumon
Trowa Barton - Gundam WingRowan - Trigun
Youko Kurama - Yuu Yuu Hakusho
Farfarello - Weiß KreuzSeraphita - Angel Sanctuary
Folken Fanel - Tenkuu no EscaflowneKing Kashue - Record of Lodoss (TV)
Childman Powderfield - Majutsushi Orphen
Hijikata Toshizo - Peace Meaker Kurogane
Hayama Akito - Kodomo no Omocha
Kagibara Tetsuya - Fushigi YuugiNeya MichikoMonou Fuuma - X
Sesshoumaru - Inu-Yasha
Yuki - Master of MosquitonNogami YukanaAsakawa Yuriko - Weiß Kreuz
Barnette Orangelo - Vandread
Monou Saya - X
Tot - Weiß KreuzSuzuhara Natsumi - Tenshi ni Narumon
Nekoi Yuzuriha - X
Spark - Record of Lodoss (TV)Mudo Setsuna - Angel Sanctuary
Cayman - GetBackersAki - Recca no Honoo
Ikari Shinji - Neon Genesis Evangelion
Princess Emerald - Magic Knight Rayearth
Eagle - Magic Knight Rayearth
Minami Shuichi (Kurama) - Yuu Yuu Hakusho
Gaddes - Tenkuu no EscaflowneOhtani IkueHanabishi Shigeo - Recca no Honoo
Ruka-chan - Tenshi ni NarumonOhtsuka AkioPikachuu - Pokemon
Guni - Nightwalker
Chibi Signal - Twin Signal
Batanen-sempai - Hyper PoliceGaou Fanel - Tenkuu no Escaflowne
Minowa Minoru - Mahou Tsukai Tai!
Udoh Jin'e - Rurouni Kenshin
Hanabishi Recca - Recca no Honoo
Brad Crawford - Weiß KreuzTreize Krushrenada - Gundam Wing
Kurei - Recca no Honoo
Akatsuki Nagai - Martian Successor Nadesico
Hartia - Majutsushi Orphen
Sohma Shigure - Fruits Basket
Nishikiori Issei - Please Save My Earth
Onosaka Masaya
Vash the Stampede - TrigunTakakura Takeo - Mahou Tsukai Tai!
Niisan - Twin Signal
Alexiel - Angel SanctuarySakuma ReiKuwabara Shizuru - Yuu Yuu Hakusho
Ryoko - Tenchi Muyo
Ohtori Kanae - Shoujo Kakumei Utena
Arshesh Ney - Bastard!!Miyama Mizuha - Mahou Tsukai Tai!
Fianna - Record of Lodoss War
Shampoo - Ranma 1/2
Naoe Nagi - Weiß KreuzEram - Arslan Senki
Shima Tetsuo - Akira
Guru Clef - Magic Knight Rayearth
Sakaguchi Hajime - Please Save My Earth
Urameshi Yuusuke - Yuu Yuu Hakusho
Van Fanel - Tenkuu no EscaflowneShirou Kamui - X
Daigohji Gai - Martian Successor Nadesico
Hidaka Ken - Weiß Kreuz
Sohma Kyou - Fruits Basket
Kouji - Fushigi Yuugi
Chichiri - Fushigi Yuugi
Duo Maxwell - Gundam WingLegato Bluesummers - Trigun
Knight - Weiß Kreuz: Glühen
Asagi Shougo - X
Watari Yutaka - Yami no Matsuei
Toboe - Wolf's RainShinohara Emi
Kagero - Juubei NinpuchoMokuren - Please Save My Earth
Matsunaga Yayoi - Nightwalker
Daitokuji B-Ko - Project A-ko
Kishyuu Arashi - X the Movie
Narsus - Arslan SenkiShiratori YuriLarva - Vampire Princess Miyu
Zongi - Tenkuu no Escaflowne
Princess Charlotte - BerserkYukina - Yuu Yuu Hakusho
Wakaba-chan - Yami no Matsuei
Sanjou Tsubame - Rurouni Kenshin
Tune Yung - Megami Kouhousei
Elara - Twin Signal
Sakaguchi Arisa - Please Save My Earth
Sohma Hatsuharu - Fruits BasketShiogami/Jigumi - Jikuu Tenshou Nazca
Hige - Wolf's Rain
Suzukaze Mayo
Himura Kenshin - Rurouni Kenshin
Miura Kyoji - Jikuu Tenshou NazcaSuzuoki HirotakaKamui - X TV
Fuge no Maya - Saint Beast
Saitoh Hajime - Rurouni KenshinTakayama MinamiKuno Tatewaki - Ranma 1/2
Dilandau Albatou - Tenkuu no EscaflownePrince Chid - Tenkuu no Escaflowne
Mukuro - Yuu Yuu Hakusho
Tendo Nabiki - Ranma 1/2
Jeanie - Mahou Senshi Riui
Ascot - Magic Knight Rayearth
Shiiris - Record of Lodoss OVA
Minase Hijiri - Yami no Matsuei
Aoki Seiichirou - XCain - Nighwalker
Ishijima Domon - Recca no HonouTominaga MiinaTomo - Fushigi Yuugi
Dobashi Daisuke - Please Save My Earth
Takeda Kanryu - Rurouni Kenshin
Myojin Yahiko - Rurouni KenshinTouma YumiSohma Ritsu - Fruits Basket
Deedlit - Record of LodossTsujitani KoujiHongo Yui - Fushigi Yuugi
Sylpheel - Slayers
Miroku - Inu-YashaTsuru HiromiJajuka - Tenkuu no Escaflowne
Hiroshi - Ranma 1/2
Camille Inaho Carmilla - Master of Mosquiton"Derringer" Meryl Strife - Trigun
Seguchi Mika - Gravitation
Kuonji Ukyou - Ranma 1/2
Sagara Sanosuke - Rurouni KenshinWakamoto NorioKatou Yue - Angel Sanctuary
Ichimura Tatsunosuke - Peace Maker Kurogane
Tenkawa Akito - Martian Successor Nadesico
Amiboshi and Suboshi - Fushigi Yuugi
Vicious - Cowboy BebopYajima AkikoUtsutsu Mujuuro - Juubei Ninpucho
Taishakuten - RG Veda
Woodchuck - Record of Lodoss (OVA)
Gambino - Berserk
Dorothy Waynewright - The Big ORickelt - Berserk
Relena Peacecraft - Gundam Wing
Kaji Ryouji - Neon Genesis EvangelionSpike Spiegel - Cowboy Bebop
Arslan - Heroic Legend of ArslanInuyasha - Inuyasha
Kasuma Haruhiko - Please Save My Earth
Sakuma Ryuichi - Gravitation
Nagakura Shinpachi - Peace Maker Kurogane
Rokuta - Juuni Kokki
Sena - Weiß Kreuz: Glühen
Sumeragi Subaru - Tokyo Babylon
Yamamoto Kouji
Hanzawa Rui - Hana Yori Dango
Ferio - Magic Knight RayearthShido Tatsuhiko - Nightwalker
Geo Metro - Magic Knight Rayearth
Dark Schneider - Bastard!!Gieve - Heroic Legend of Arslan
Wataru - Wind Named Amnesia
Shinomori Aoshi - Rurouni KenshinYokoyama Chisa
Lucrezia Noin - Gundam WingYoshida KonamiSasami, Tsunami - Tenchi Muyo
Ryoko - Nadesico
Sheila-hime - Bastard!!Yoshino HiroyukiTatsuko (referee) - Recca no Honoo
Ryuuzaki Umi - Magic Knight Rayearth
Tokai Hibiki - VandreadYukino SatsukiByakko no Gai - Saint Beast
Clay Cliff Fortran - Megami Kouhousei
Milly Thompson - TrigunHirugashi Kagome - Inu Yasha
Tina Foster - Ai Yori Aoshi
Tsukiyono Omi - Weiß KreuzMikage Mahoro - Samurai: Hunt for the Sword
Signal - Twin Signal
Check out the Seiyuu Resource . There is also Hitoshi Doi's Anime Page and a French site called Animes et Mangas . They are all excellent resources for the seiyuu search.
A personal site is Gryvon's Anime Page . It has a lot of minor roles.
Another really good site is the Voice Actor Page. It has a LOT of information, although some of it is not necessarily accurate. It also has information on dub actors for English, and dubs of American movies and shows in other languages (mostly Japanese, from what I can see). Beware of incorrect information though, since it all seems to be submitted by viewers.
A very meticulous and hopefully accurate list of seiyuu and shows can be found on the Anime News Network.
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